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核聚变与等离子体物理 ›› 2008, Vol. 28 ›› Issue (2): 187-192.

• 等离子体应用 • 上一篇    

非平衡等离子体水处理器的优化设计及性能评价

张延宗1,郑经堂1,王广昌2,桑玉全1, 3,陈宏刚3   

  1. 张延宗1,郑经堂1,王广昌2,桑玉全1, 3,陈宏刚3
  • 收稿日期:2007-03-05 修回日期:2007-09-12 出版日期:2008-06-15 发布日期:2011-02-21
  • 作者简介:张延宗(1968-),男,山东临邑人,博士研究生,主要从事于非平衡等离子体应用于环境污染治理方面的研究。
  • 基金资助:

    国家自然科学基金资助项目(20576079,20776159)

Optimization design and performance evaluation of non-equilibrium plasma reactor for waste water treatment

ZHANG Yan-zong1, ZHENG Jing-tang1, WANG Guang-chang2,SANG Yu-quan1, 3, CHEN Hong-gang1   

  1. (1. State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Dongying 257061;2. Research Institute of Chemical Defence, Beijing 102205;3. Environment Monitoring Station of Shengli Oilfield Company Limited, Dongying 257061)
  • Received:2007-03-05 Revised:2007-09-12 Online:2008-06-15 Published:2011-02-21

摘要:

在正交实验和单因素实验的基础上,对非平衡等离子体水处理反应器的整体结构进行了优化设计,并对优化后反应器的性能进行了定性评价。正交实验结果表明,影响降解效率的因素为气高、液高和气体流量。针高度为4mm电极间距17mm、气体流量为96L·h-1时甲基橙的降解效果最佳。用40不锈钢网作地电极,采用正脉冲放电能提高降解效率,预处理溶液中放置不锈钢阻挡网有助于提高臭氧的利用率。降解效率和COD去除率随溶液初始浓度的增加而降低,但相同时间内有机污染物的绝对去除量增加,重复实验表明实验误差小于3.5%

关键词: 非平衡等离子体, 反应器, 优化设计, 性能评价

Abstract:

The monolithic construction of the non-equilibrium plasma reactor is optimized and the performance of the reactor was estimated on the basis of orthogonal and single factor experiments. The experimental results show that the primary and secondary factor influencing degradation efficiency is the height of air layer, the height of aqueous solution and the gas flow, respectively. The best result is obtained when the needles length in water is 5mm, the electrode gap is 17mm and the gas flow is 96L•h-1. The degradation efficiency can be improved when positive pulse was applied to the high voltage electrode and the ground electrode was made of stainless steel mesh with mesh size of 0.42mm. The design, fixed the stainless steel mesh barriers in the solution for pretreatment, increases the utilization factor of ozone. Although the degradation efficiency and COD removal are decreased with the increase of initial solution concentration, the absolute conversion amount of organic contamination increases in the same time. The repeated tests indicate that the experiment error is less than 3.5%.

Key words: Non-equilibrium plasma, Reactor, Optimization design, Performance evaluation

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